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I've lately been obsessing over the Persona series social linking arcana and despite we got arcana break RIGs with NPCs tarot, I feel like a persona version would sound fitting for some.

0: The Fool-Gaians (Protagonist:Gino Gambino) ((initial persona: Shiki-Ouji, Ultimate Persona: Loki)
1: The Magician-Liam (Initial Persona: Dis, Ultimate Persona: Surt)
2: The Priestess-Meredith
3: The Empress-Rosamund
4: The Emperor- LadyHands (Initial persona:Okuninushi , Ultimate Persona:Odin)
5: The Hierophant-Edmund (Initial Persona: Yama , Ultimate Persona:Hachiman )
6: The Lovers-Sasha
7: The Chariot-Sam
8: Justice-Ciro (Initial Persona: Power, Ultimate Persona: Dominion)
9: The Hermit-Ian Von Helson
10: Fortune-Brennivin (Initial Persona: Fortuna , Ultimate Persona: Clotho)
11: Strength-Principal Mills
12: The Hanged Man-Kanoko
13: Death-Stein
14: Temperance-Cordell
15: The Devil-Vanessa
16: The Tower-Azrael (Initial Persona: Cu Chulainne, Ultimate Persona: Amatsu Mikaboshi)
17 The Star-Marius (Initial Persona: Hoenir, Ultimate Persona: Kartikeya)
18: The Moon-Sentinel (initial Persona: Alraune, Ultimate Persona: Salome)
19: The Sun-Meili
20: Judgment-Nyx's Arrival
21: The world/Universe-Ambition
Jester card-Monsieur Loyal
Aeon Card-Ami Satomora (Persona: Sati)
Hunger card-Nyx

Feel free to add more here. And here's the link and click on the arcana links if you don't know which would fit which NPC.

http://megamitensei.wikia.com/wiki/Arcana